American Association for Aerosol Research - Abstract Submission

AAAR 35th Annual Conference
October 17 - October 21, 2016
Oregon Convention Center
Portland, Oregon, USA

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Characterization of the Aqueous Oxidation of Glyoxal and Methylglyoxal in the Presence of Salts Using a Quartz Crystal Microbalance

Hannah Holst, Alvin Burrows, Maeve Ryan, CHRISTEN STROLLO, CSBSJU

     Abstract Number: 520
     Working Group: Aerosol Chemistry

Abstract
The focus of this project is to determine the physical properties of products formed from the aqueous phase reactions of glyoxal with hydroxyl radicals. Glyoxal and methylglyoxal are the most abundant dicarbonyls in the atmosphere and contribute to the formation of secondary organic aerosol (SOA). A quartz crystal microbalance (QCM) equipped with a humidity controlled flow cell is used to measure the deliquescence of a variety of reaction solutions. Solutions are aspirated onto the quartz crystal and subsequently dried, then exposed to increasing humidity. Understanding SOA in aqueous aerosols has the potential to eliminate the gap between predicted and measured SOA formed from gas-partitioning. Here, we describe the specific characteristics of the aqueous reaction of dicarbonyls commonly present in the atmosphere as well as the effect of the presence of salts has on the deliquescence of the resultant solutions.